O Espião do Chapéu Verde
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Robert VaughnNapoleon Solo
David McCallumIllya Kuryakin
Jack PalanceLouis Strago
Janet LeighMiss Diketon
Eduardo CiannelliArturo 'Fingers' Stilletto
Allen JenkinsEnzo 'Pretty' Stilletto
Jack La RueFederico 'Feet' Stilletto
Leo G. CarrollAlexander Waverly
Joan BlondellMrs. 'Fingers' Stilletto
Ludwig DonathDr. Heinrich von Kronen
Will KuluvaMr. Thaler, Thrush Boss
Letícia RománPia Monteri- Penny SantonGrandma Monteri
Frank PugliaPadre
Vincent BeckBenjamin Luger
Maxie Rosenbloom'Crunch' Battaglia
Vince Barnett'Scissors'
Elisha Cook Jr.Arnold
James AlmanzarThrush Captain- Clarke GordonThrush Officer
Jesslyn FaxMrs. Feinberg- Jimmy BatesBoy
- David RenardDonkey Man
Sharyn HillyerMiss Gorgeous
Anne CaprileMiss Diketon (french voice) (sem créditos)
Leoda Richards